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Journal Articles

Preliminary analysis of randomized configuration patterns in modified STACY core

Shiba, Shigeki*; Iwahashi, Daiki*; Okawa, Tsuyoshi*; Gunji, Satoshi; Izawa, Kazuhiko; Suyama, Kenya

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 9 Pages, 2023/05

The Nuclear Regulation Authority (NRA) has tackled the experimental approach for determining the criticality of pseudo-fuel debris plausibly simulating actual fuel debris since 2014, collaborating with the Japan Atomic Energy Agency. To elucidate the characteristics of the pseudo-fuel debris, the Japan Atomic Energy Agency modified the STACY (STAtic experiment Critical facilitY) to conduct critical experiments simulating fuel debris. Thus, we proposed three types of modified STACY core configurations. In critical experiments in the modified STACY core, it is important to judge whether the proposed modified STACY core configurations are representative of molten core-concrete interaction debris or not. In this study, we built pseudo-fuel debris models considering a volume ratio of pseudo-fuel debris to moderation (V$$_{m}$$/V$$_{f}$$) and calculated uncertainty-based similarity values (C$$_k$$) between the modified STACY core configurations and pseudo-fuel debris models using Tools for Sensitivity and Uncertainty Analysis Methodology Implementation-Indices and Parameters (TSUNAMI-IP) in SCALE 6.2. Consequently, the modified STACY core configuration loading structure rods we proposed completely resulted in high similarity to the pseudo-fuel debris models through V$$_m$$/V$$_f$$ values. The main contributions to C$$_k$$ values were $$^{235}$$U $$bar{nu}$$, $$^{235}$$U $$chi$$, and $$^{56}$$Fe (n,$$gamma$$), except for the pseudo-fuel debris model, including extremely high concrete components.

JAEA Reports

Thermodynamic Date for Predicting Concentrations of Pu(III), Am(III), and Cm(III) in Geologic Environments

Rai, D.*; Rao, L.*; Weger, H. T.*; GREGORY R.CHOPPI*; Yui, Mikazu

JNC TN8400 99-010, 95 Pages, 1999/01

JNC-TN8400-99-010.pdf:3.88MB

This report provides thermodynamic data for predicting concentrations of Pu(III), Am(III), and Cm(III) in geologic environments, and contributes to an integration of the JNC chemical thermodynamic database, JNC-TDB (previously PNC-TDB), for the performance analysis of geological isolation system for high-level radioactive wastes. Thermodynamic data for the formation of complexes or compounds with hydroxide, chloride, fluoride, carbonate, nitrate, sulfate and phosphate are discussed in this report. Where data for specific actinide(III) species are lacking, the data were selected based on chemical analogy to other trivalent actinides. In this study, the Pitzer ion-interaction model is mainly used to extrapolate thermodynamic constants to zero ionic strength at 25$$^{circ}$$C.

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